Coherent Sensing

Welcome to our group website!

Our work is dedicated to high resolution spectroscopy with frequency combs and coherent sensing. We use ultrashort laser pulses on the femtosecond time scale to learn more about the optical properties and transient dynamics of atoms and molecules, so far mostly in the gas phase. Recently, we have extended our research focus to applications of photochemical and biophysical relevance.

Coherent Sensing Group in May 2026.
From left to right: Elias Ehl, Birgitta Schultze-Bernhardt, Christoph Gruber, Mithun Pal, Johannes Spendier
(missing on the photo: Armin Speletz).
Coherent Sensing Group with the group’s mobile field spectrometer operating in the visible and ultraviolet spectral region, May 2026. From left to right: Armin Speletz, Johannes Spendier, Elias Ehl,
Birgitta Schultze-Bernhardt, Mithun Pal, Christoph Gruber.

Research

1. Dual comb spectroscopy in different spectral regions

Dual Comb Spectroscopy combines high spectral resolution with broad spectral coverage and short measurement times. In the recent years, this spectroscopic method has proven its capabilities in molecular spectroscopy in different spectral regions ranging from the visible across the infrared spectral region into the THz domain, see for example [1-3]. We are currently expanding dual comb spectroscopy for different applications ranging from the detection of unknown gas mixtures such as our complex atmosphere to Raman spectroscopy for the examination of biophysical samples [2].

2. Electronic Fingerprint Spectroscopy

So far our knowledge about (extreme) UV characteristics of atomic and molecular gasses and condensed matter is scarce due to the lack of readily available laser sources in this spectral region. Especially high resolution spectroscopic studies with an advanced resolving power on the order of 105 and 106 still have to be performed at synchrotron sources that are only restrictedly accessible. In the recent years, the high power laser technology has prospered such that table top high photon flux (X)UV sources with high repetition rates become possible not only with enhancement cavities [4] but also in single pass geometry. However, laboratory (X)UV spectroscopic studies are still limited by conventional grating spectrometers that typically provide a resolving power on the order of 103 [5,6].  At the IEP, we are currently developing UV dual comb spectroscopy that will enable unparalleled resoling powers of 10-7 and beyond outperforming synchrotron-based spectrometers by at least one order of magnitude and grating based XUV spectrometers by more than four orders of magnitude [7].

Recently, we have developed a mobile dual comb spectrometer operating in the visible spectral region that we used for field monitoring of NO2 in the city of Graz [8]. The world’s first broadband NUV dual comb spectrometer enabled the simultaneous detection of rovibrational states in formaldehyde and real time monitoring of this environmentally highly relevant pollution gas [9]. Our subsequent spectrometer platform could achieve the highest dual comb quality factor to date reported in the UV combining advanced resolving power of 106, short acquisition times (500 ms) with high signal to noise ratios (> 250) and broad spectral coverage (> 10 THz). With this, the rovibrational substructure of the formaldehyde absorption spectrum in the atmospherically relevant UV region could be examined with unprecedented detail and sensitivity unravelling so far experimentally unobserved transitions [10].

Figure 1: Comparison of ultraviolet absorption cross section measurements in formaldehyde a DCS absorption cross section spectrum of HCHO (blue, above the abscissa) compared to previous measurements (see details in [10]). The spectrum was recorded at T = 294 K, p(HCHO) = 90 mbar, with an optical path length of 310 cm and an acquisition time of 0.5 s. & f The strong absorption features of both traces agree qualitatively but display minor differences in the line positions. & g The DCS spectrum has an up to 20 times lower noise level, despite a substantially shorter acquisition time (0.5 s for DCS versus 60 min). d, e & h, i For frequencies above 853 THz, the DCS trace resolves the rovibronic lines for the first time. The mean relative absorption cross section uncertainty amounts to 7.2%. Figure taken from [10].

Further recent works of the coherent sensing group:

  • Streaming Dual Comb Spectroscopy in Real-Time: Eber, A., Gruber, C., Schultze, M., Bernhardt, B., Ossiander, M., Streaming self-corrected dual-comb spectrometer. Optics Express 33: 35314–35325 (2025), https://doi.org/10.1364/OE.569404
  • Systematic Comparison of dual comb spectroscopy with different repetition rate regimes: NIR/VIS dual-comb spectroscopy comparing high and low repetition rate regimes. A Eber, M Pal, L Fürst, E Hruska, C Gruber, M Ossiander, B Bernhardt; Laser & Photonics Reviews, e02713 (2026)
     
  • Together with the Leonahrd Grill Group, Uni Graz: : Switching Azobenzene Derivatives on Au(111) Analyzed by Advanced Computer Vision Methods, Matthew James Timm; Alexander Eber; Emily Hruska; Stefan Hecht; Leonhard Grill; Birgitta Bernhardt, Surface Science, 122971 (2026) https://doi.org/10.1016/j.susc.2026.122971
     
  • Resonant dispersive-wave frequency comb generation: Kirchner, A., A. Eber, L. Fürst, E. Hruska, M. H. Frosz, F. Tani, and B. Bernhardt (2025). Ultra-broadband UV/VIS spectroscopy enabled by resonant dispersive wave emission of a frequency comb, Optics Express, 33, 7005–7015 (2025), https://doi.org/10.1364/OE.546751

This research is funded the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program (grant agreement no. 947288), by the Austrian Science Fund FWF START program (grant agreement no. Y1254N) and the NAWI Graz infrastructure funding program.

Recent news

June 3rd 2026

TU Graz Physicist Presents Mobile Device for High-Precision Measurement of Air Pollutants

The UV dual-comb spectrometer detects harmful gases with unrivalled accuracy and sensitivity. The compact design allows mobile use for monitoring air quality with a range of several kilometres.

TU Graz News

V.l.: Rolf Breinbauer, Birgitta Schultze-Bernhardt, Clemens Hofmann und Mithun Pal stehen am UV-Breitband-Spektrometer. Bildquelle: Wolf – TU Graz

March 20th 2026

New Paper Out!

Our frequency combs have entered the fascinating world of Surface Science!

So far, our combs enabled "just" superior spectral resolution.  In our most recent work, one of our combs helped to shed light onto the complex switching behavior of azobenzene molecules  - with single molecule resolution. Special thanks go to our Coherent Sensing team mate Robert di Vora for his powerful computer vision algorithm and to Matthew Timm and Leonhard Grill for introducing us to their STM realm!

Check out our joint publication in Surface Science: https://doi.org/10.1016/j.susc.2026.122971

#FrequencyCombs #ERCStartingGrant #CoherentSensing

January 15th 2026

New Paper Out!

Our work on NIR/VIS dual comb spectroscopy with low and high repetition rate regimes is published in Lasers & Photonics Reviews!
In this paper, we have compared two dual comb systems operating at 80 MHz and 1 GHz repetition rates. Both have their advantages - depending on the envisioned applications

check out the details here:

NIR/VIS Dual‐Comb Spectroscopy Comparing High and Low Repetition Rate Regimes - Eber - Laser & Photonics Reviews - Wiley Online Library

1st November 2025

Johannes SPENDIER joins our team

 

Herzlich Willkommen, Johannes!

12th October 2025

Our research at FÄKT!

This time, we were visited by Julia and the FÄKT team and had a great time showcasing our lasers in action!
How do our measurements actually work, and what are we discovering about the air quality in Graz?

FÄKT is a science communication project by the Austrian Academy of Sciences (ÖAW), aimed especially at a young audience. Curious? Then check out the result from Graz here:

14th July 2025

Measuring Air Pollutants in Real Time: ERC Proof of Concept Grant for TU Graz Physicist

Birgitta Schultze-Bernhardt receives funding from the European Research Council for the development of a portable device that measures several pollutants simultaneously in a fraction of a second.
TUG Pressemitteilung

Birgitta Schultze-Bernhardt, TU Graz
© Lunghammer

June 18th 2025

RIGOROSUM

Adrian KIRCHNER
Agile frequency upconversion for ultra-broadband dual comb spectroscopy across the visible and ultraviolet spectral regions

Adrian Kirchner successfully defended his doctoral thesis „ Agile frequency upconversion for ultra-broadband dual comb spectroscopy across the visible and ultraviolet spectral regions“ on June 18th 2025. We could invite our collaboration partner Prof. Arnaud Mussot, University of Lille, to Graz as second reviewer who is an expert on EOM frequency combs including all-fiber frequency agile triple-frequency comb light sources.

Congratulations, Adrian!

May 5th 2025

New Paper Out!

Our work on a phase locked feed forward stabilization scheme for dual comb spectroscopy is published in Ultrafast Science Journal.

It improves our existing IR/VIS dual comb spectrometer operated at 80 MHz in terms of spectral resolution (three orders of magnitude) and sensitivity (one order of magnitude). For our NO2 field measurements, this means an improved detection limit down to 1 ppb!

Check it out:

Phase-Locked Feed-Forward Stabilization for Dual-Comb Spectroscopy | Ultrafast Science

Special thanks go to Marcus Ossiander for the inspiring team work!

If you are interested in older news, visit our "News Archive"!

Selected Publications

[1] B. Bernhardt, A. Ozawa, P. Jacquet, M. Jacquey, Y., T. Udem, R. Holzwarth, G. Guelachvili, T. W. Hänsch and N. Picqué, Cavity-enhanced dual-comb spectroscopy, Nature Photonics 4, 55-57 (2009)
https://doi.org/10.1038/nphoton.2009.217

[2] T. Ideguchi, S. Holzner, B. Bernhardt, G. Guelachvili, N. Picqué and T. W. Hänsch, Coherent Raman spectro-imaging with laser frequency combs, Nature 502, 355 (2013)
https://doi.org/10.1038/nature12607

[3] T. Ideguchi, B. Bernhardt, G. Guelachvili, T.W. Hänsch and N. Picqué, Raman-induced Kerr-effect dual-comb spectroscopy, Optics Letters, Vol. 37, 4498 (2012)
https://doi.org/10.1364/OL.37.004498

[4] B. Bernhardt, A. Ozawa, A. Vernaleken, I. Pupeza, J. Kaster, Y. Kobayashi, R. Holzwarth E. Fill, F. Krausz, T. W. Hänsch, and Th. Udem, Vacuum ultraviolet frequency combs generated by a femtosecond enhancement cavity in the visible, Optics Letters 4, 503 (2012)
https://doi.org/10.1364/OL.37.000503

[5] B. Bernhardt, A. R. Beck, X. Li, E. R. Warrick, M. J. Bell, D. J. Haxton, C. W. McCurdy, D. M. Neumark and S. R. Leone, High-spectral-resolution attosecond absorption spectroscopy of autoionization in xenon, Physical Review A 89, 023408 (2014)
https://doi.org/10.1103/PhysRevA.89.023408

[6] K. Hütten, M. Mittermair, S. Stock, R. Beerwerth, V. Shirvanyan, J. Riemensberger, A. Duensing, R. Heider, M. Wagner, A. Guggenmos, S. Fritzsche, N. M. Kabachnik, R. Kienberger and B. Bernhardt, Ultrafast Quantum Control of Ionization Dynamics, Nature Communications 9, 719 (2018)
https://doi.org/10.1038/s41467-018-03122-1

[7] V. Schuster, C. Liu, R. Klas, P. Dominguez, J. Rothhardt, J. Limpert, and B. Bernhardt, Ultraviolet dual comb spectroscopy: a roadmap, Optics Express 29, Issue 14, 21859-21875 (2021)
https://doi.org/10.1364/OE.424940

[8] A. Eber, et al., Coherent field sensing of nitrogen dioxide, Opt Express 32, 6575 (2024)
https://doi.org/10.1364/OE.513523

[9] Fürst, Lukas, et al., Broadband near-ultraviolet dual comb spectroscopy, Optica 11.4, 471-477 (2024)
https://doi.org/10.1364/OPTICA.516783

[10] L. Fürst, M. Pal, A. Eber, E. Hruska, C. Hofmann, IE. Gordon, M. Schultze, R. Breinbauer and B. Bernhardt, Free-running ultraviolet dual comb spectroscopy enabling absolute electronic fingerprinting, PhotoniX 7 (1), 33 (2026)
https://doi.org/10.1186/s43074-026-00250-6

Lab Tour & Fotos

Visit our lab virtually via YouTube (in German):

Lab Fotos

[-] Dual Comb Lab
[-] Dual Comb Lab
[-] Dual Comb Spectrometer operating in the visible spectral region
[-] Iodine Cell
[-] NIR-VIS Dual Comb Spectrometer

Alumni and their last known whereabouts

Dr. Adrian Kirchner, K2 Photonics
Dr. Emily Hruska, Wiley-VCH Verlag
Dr. Alexander Eber, Anton Paar GmbH
Dr. Lukas Fürst, Heidenhain GmbH
M. Sc. Florian Lindorfer
Dr. Florian Siegrist, Anton Parr GmbH

Funding

All images © TU Graz/Institute of Experimental Physics
Contact
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Institut of Experimental Physics
Graz University of Technology
Petersgasse 16
8010 Graz
Austria

Group Leader
Birgitta BERNHARDT,
Univ.-Prof. Dipl.-Phys. (Univ.) Dr.rer.nat.

Tel.: +43 (0) 316 / 873 - 8663
Fax: +43 (0) 316 / 873 - 8655

bernhardt@tugraz.at

Group Members
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Univ.-Prof. Dipl.-Phys. (Univ.) Dr.rer.nat. Birgitta BERNHARDT
Curriculum Vitae
bernhardt@tugraz.at
+43 (316) 873-8663


BSc DI Armin SPELETZ
armin.speletznoSpam@tugraz.at
+43(316)873-8928

 

BSc MSc Ph D. Mithun PAL
mithun.palnoSpam@tugraz.at
+43(316)873-8640
 
   


BSc MSc Elias EHL
elias.ehlnoSpam@tugraz.at
+43 (316) 873-8662

 
 
MSc Christoph GRUBER
christoph.grubernoSpam@tugraz.at
+43 (316) 873-8167
 
 
BSc Johannes SPENDIER
johannes.spendier@stundent.
tugraz.at

+43 (316) 873-8147
Links
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